SYNTHESIS AND REACTIONS OF UNSYMMETRICAL DISULFIDES AND DISULFONES. RING-CLOSURE REACTIONS OF BETA-ARYLETHYL DISULFIDES.

Abstract

Bis-o-biphenylyl disulfide was found to cyclize to dibenzothiophene in excellent yield when treated with iodine in refluxing ethylene glycol. Under similar conditions, bis-beta-2-naphthylethyl disulfide gave a poor yield of 2,3-dihydronaphtho-(1,2-b)thiophene. Using excess iodine, the product is mainly naphtho(1,2-b) thiophene. These products were identified by conversion to picrates and oxidation to naphtho(1,2-b)thiophene-1,1dioxide. Bis-1-phenylcyclohexyl disulfide, prepared from X-acetyl-2-phenylcyclo-hexanethiol, could not be cyclized under the influence of iodine in ethylene glycol. A large percentage of the disulfide was recovered, along with some biphenyl. (Author)

Document Details

Document Type
Technical Report
Publication Date
Apr 25, 1961
Accession Number
AD0614690

Entities

People

  • B. G. Heaton
  • E. Campaigne

Organizations

  • Indiana University Bloomington

Tags

DTIC Thesaurus Topics

  • Acyclic Hydrocarbons
  • Alkenes
  • Biphenyl
  • Chemical Compounds
  • Conversion
  • Ethylene Glycol
  • Ethylenes
  • Glycols
  • Hydrocarbons
  • Organic Compounds
  • Oxidation

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry