THE USE OF MATHEMATICAL PROGRAMMING IN THE CALCULATION OF ATOMIC WAVE FUNCTIONS.
Abstract
The observed energy levels for Silicon + 3 have been fit by adding a polarisation term to the potential of the Hartree-Fock equation in a manner first used by Douglas. The resulting wave functions were used to calculate transition integrals for the allowed transitions and compared with the results using no polarisation term; the differences were of the order of a few percent. Results of calculations done on Silicon + 2 to determine the form of the polarisation term for the two-electron case are reported. The isoelectronic sequence from Sodium to Argon + 7 was examined to determine the possibility of predicting polarisation functions without knowledge of observed energy levels; difficulties in making the prediction are discussed. Changes in the numerical procedure for solving the Hartree-Fock equations are presented along with changes in the program for adding the polarisation term. (Author)
Document Details
- Document Type
- Technical Report
- Publication Date
- Mar 01, 1965
- Accession Number
- AD0617705
Entities
People
- D. F. Mayers
- F. O'brien