OPTICAL VIBRATION SPECTRA OF SOLIDS.

Abstract

The infrared reflection and/or transmission spectra of CdS, ZnS, ZnO, BN, NiO, CoO, and their mixed crystals, MnO, Al2O3, Mg(OH)2 and Cu2S are reported at one or more temperatures. The Raman spectrum of ZnO is also reported. The experimental investigations also included the study of crystal field spectra of Ni(2+), Co(2+) and Mn(2+) in their respective monoxides. The infrared and the ultraviolet absorption by U-centers in alkali halides was studied and interpreted in terms of localized virational modes of the impurity centers. Theoretical investigations include discussions on: (i) The trends in the characteristic phonon frequencies of the II-VI compounds, (ii) the assignment of the multiphonon infrared absorption in GaAs using the space group selection rules, (iii) the validity of the LyddaneSachs-Teller relationship at long wavelengths, (iv) the combination of the lattice modes with the internal modes in a crystal containing polyatomic groups, and (v) the Gruneisen parameter for long wavelength optical modes in ionic crystals. (Author)

Document Details

Document Type
Technical Report
Publication Date
Aug 03, 1965
Accession Number
AD0626595

Entities

People

  • Shashanka S. Mitra

Organizations

  • IIT Research Institute

Tags

DTIC Thesaurus Topics

  • Absorption
  • Crystal Lattice Vibrations
  • Crystal Lattices
  • Crystal Structure
  • Crystals
  • Frequency
  • Gruneisen Parameter
  • Ionic Crystals
  • Long Wavelengths
  • Raman Spectra
  • Spectra

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.
  • Spectroscopy.

Technology Areas

  • Space