STUDYING VULCANIZATION OF FLUOROCOPOLYMERS WITH POLYAMINES BY INFRARED SPECTROSCOPY METHOD,

Abstract

It was found that the vulcanization of a hexafluoropropylene-vinylidene fluoride with hexamethylenediamine (HMDA) results in the formation of a HMDAhydrofluoride salt (as a result of dehydrofluorination of the copolymer) and the formation of double bonds in the polymer chain which, in turn, join with a portion of the HMDA to form C-N and C=N bonds. In the presence of MgO the same bonds are formed, but without the formation of the HMDA-hydrofluoride. Heating the mixture of the copolymer and HMDA-HF results in the dehydrofluorination of the latter compound, making additional HMDA available for bond formation. The separated HF, however, tends to disrupt the C=N bonds. The susceptibility of these bonds may be the primary cause of the relatively low heat and acid resistance of fluoro-copolymers vulcanized with polyamines.

Document Details

Document Type
Technical Report
Publication Date
Dec 21, 1965
Accession Number
AD0627005

Entities

People

  • A. S. Novikov
  • F. A. Galil-oglii

Organizations

  • National Air and Space Intelligence Center

Tags

DTIC Thesaurus Topics

  • Amines
  • Chemical Compounds
  • Copolymers
  • Fluorides
  • Infrared Spectroscopy
  • Polymers
  • Resistance
  • Spectroscopy
  • Ultraviolet Spectroscopy
  • Vulcanization

Readers

  • Polymer Science and Engineering.
  • Powder metallurgy of Titanium alloys.

Technology Areas

  • Microelectronics