MICROWAVE SPECTRUM, INTERNAL BARRIER, MOLECULAR STRUCTURE AND DIPOLE MOMENT OF DISILANYL FLUORIDE.

Abstract

The microwave spectra of five isotopic species of disilanyl fluoride (Si2H5F) were studied in the region 12-38 Gc/sec. Several of the ground state transitions are split into doublets, some into triplets, due to the coupling of internal and overall rotation. Analysis of the splittings gives a barrier value V-3 = 1048 plus or minus 40 cal/mole. Rotational constants were determined for molecules containing silicon-28, -29 and -30 isotopes in each positions, and were used to calculate the structure. Stark effect measurements yield mu-A = 0.934 D, mu-B = 0.850 D and a total dipole moment mu = 1.26 plus or minus 0.01 D inclined at an angle of 10 degrees to the SiF bond. (Author)

Document Details

Document Type
Technical Report
Publication Date
Jan 01, 1965
Accession Number
AD0628118

Entities

People

  • A. Peter Cox
  • Ravi Varma

Tags

DTIC Thesaurus Topics

  • Couplings
  • Diffraction
  • Dipole Moments
  • Electromagnetic Spectra
  • Fluorides
  • Ground State
  • Measurement
  • Microwaves
  • Molecular Structure
  • Molecules
  • Rotation
  • Spectra
  • Splitting
  • Stark Effect
  • Transitions
  • Wave Phenomena

Fields of Study

  • Physics

Readers

  • Analytical Mechanics
  • Electrochemical Engineering/ Fuel Cell Technologies
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.