FAR INFRARED STUDIES OF HYDROGEN BONDING.

Abstract

Direct spectroscopic observations of the hydrogen bond stretching frequencies in the pure cresols and chlorophenols were obtained in the far infrared. Previous difficulties in making assignments were obviated by the use of the following criteria, which provide unambiguous identification of the stretching frequency: (1) disappearance of the absorption when -OCH3 is substituted for -0H; (2) absence of the band in the Raman spectrum; (3) observation of a broad asymmetric band contour. Although no generalizations may yet be drawn, there is no simple correlation between hydrogen bond streching frequency and near infrared bonded 0-H frequency shifts for these compounds. The stretching frequency of the intramolecular H-bond in o-chlorophenol is lower than those of the intermolecular hydrogen bonds in the other examples. (Author)

Document Details

Document Type
Technical Report
Publication Date
Mar 01, 1966
Accession Number
AD0632001

Entities

People

  • George E. Leroi
  • Irwin D. Kuntz Jr.
  • William J. Hurley

Tags

DTIC Thesaurus Topics

  • Absorption
  • Frequency
  • Frequency Shift
  • Hydrogen
  • Hydrogen Bonds
  • Identification
  • Observation
  • Raman Spectra
  • Spectra

Readers

  • Quantum Chemistry
  • Theoretical Analysis.