THE THERMODYNAMICS OF M-CENTER FORMATION.
Abstract
The equilibrium between F centers and M centers in additively colored KC1 was studied at temperatures between 60C and 130C. The M-center concentration at equilibrium varied approximately as the square of the F-center concentration, verifying the stoichiometric equation: 2F = M. At 60C, the equilibrium constant was 1.7 x 10 to the-19th power cu.cm. Enthalpy change = -4.1 Kcal and entropy change = -98 cal/deg, for the standard state one center cu.cm. The entropy change value agrees with that calculated from the configurational entropy, i.e., R 1n 6/N, where N is the concentration of negative ion sites. (Author)
Document Details
- Document Type
- Technical Report
- Publication Date
- Jul 10, 1966
- Accession Number
- AD0636316
Entities
People
- Allen B. Scott
- E. H. Coker
- John D. Zahrt
Organizations
- Oregon State University