HYDROTHERMAL GARNET CRYSTALS: HYDROTHERMAL CRYSTAL GROWTH OF CALCIUM ALUMINOSILICATE GARNET CONTAINING DIVALENT RARE EARTH IONS

Abstract

The aim of this research was the hydrothermal growth of single crystals of grossular garnet, Ca3Al2Si3O12, containing divalent activator ions such as Eu, Sm, Gd, Ce and Mn. Such crystals were desired as possible new laser materials with efficient pumping and high fluorescent yield characteristics. Hydrothermal processes were successfully developed for growth of synthetic grossular on seeds and have yielded good quality fully synthetic crystals up to 3 mm x 5 mm x 9 mm. Incorporation of the rare earth ions Eu, Sm and Yb into the lattice under reducing conditions was achieved, but excitation and fluorescence spectra indicated the presence of only trivalent rare earth ions in the grossular crystals.

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Document Details

Document Type
Technical Report
Publication Date
Dec 27, 1966
Accession Number
AD0646231

Entities

People

  • A. M. Taylor
  • D. W. Breck
  • E. M. Flanigen
  • N. R. Mumbach
  • R. M. Milton

Tags

Communities of Interest

  • Advanced Electronics
  • Ground and Sea Platforms
  • Weapons Technologies

DTIC Thesaurus Topics

  • Chemical Synthesis
  • Chemistry
  • Crystal Growth
  • Crystals
  • Fluorescence
  • High Pressure
  • Inorganic Chemistry
  • Materials
  • Measurement
  • Nesosilicates
  • New York
  • Rare Earth Elements
  • Silicates
  • Single Crystals
  • Spectra
  • Tectosilicates
  • Temperature Gradients

Fields of Study

  • Chemistry

Readers

  • Materials Science and Engineering.

Technology Areas

  • Directed Energy
  • Directed Energy - Pulsed-Laser Deposition