DIFFUSION STUDIES IN LEAD SULFIDE.

Abstract

The ratio of tracer diffusion coefficients, D sub Pb 210/D sub Bi 210, at 700C is independent of deviations from stoichiometry for undoped lead sulfide single crystals and crystals doped with 4 x 10 to the 18th power and 4 x 10 to the 19th power bismuth atoms and is equal to one. The addition of 4 x 10 to the 18th power atoms of bismuth to lead sulfide does not increase the diffusion coefficients of Pb210 and Bi210 for -6.7 < log p sub S2 < 0.0 at 700C. For log p sub S2 > -3.9 and at 700C the singly ionized cation vacancy is the predominant defect through which Pb210 and Bi210 diffuse and is the majority atomic defect in undoped lead sulfide and lead sulfide doped with 4 x 10 to the 18th power bismuth atoms. The addition of 4 x 10 to the 19th power atoms of bismuth increases the self-diffusion coefficients of Pb210 and Bi210 for -6.7 < log p sub S2 < 0 at 700C. (Author)

Document Details

Document Type
Technical Report
Publication Date
Jan 31, 1967
Accession Number
AD0649047

Entities

People

  • J. Bruce Wagner Jr.

Organizations

  • Northwestern University

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Coefficients
  • Crystals
  • Diffusion
  • Diffusion Coefficient
  • Single Crystals

Readers

  • Materials Science and Engineering.