ROLE OF CONDENSED-PHASE REACTIONS IN IGNITION AND DEFLAGRATION OF AMMONIUM PERCHLORATE PROPELLANTS

Abstract

The contribution of exothermic, condensed-phase reactions to ignition and deflagration of propellants is examined. Measurements of the rates of heat release, thermal diffusivity, burning rate and ignition are combined to demonstrate the role of reactions in propellants made up of powdered ammonium perchlorate and catalysts. By means of a theoretical analysis, it is found that for the propellants under study a thermal runaway in the condensed phase can account for the ignition phenomena observed. Also, at low steady-state deflagration rates the contribution of the solid-phase reactions can be demonstrated. Some of the propellants quenched during deflagration have shown the existence of a subsurface layer, which is located in a zone at which the temperature has reached the level characteristic of the crystal transition of ammonium perchlorate.

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Document Details

Document Type
Technical Report
Publication Date
May 12, 1967
Accession Number
AD0652617

Entities

People

  • Henry Wise
  • Leonard Mcculley
  • S. H. Inami

Organizations

  • SRI International

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Ammonium Perchlorate
  • Burning Rate
  • Chemical Reaction Properties
  • Chemical Reactions
  • Combustion
  • Exothermic Reactions
  • Heat Transfer
  • Ignition
  • Measurement
  • Perchlorates
  • Phase
  • Phase Transformations
  • Solid Phases
  • Steady State
  • Thermal Diffusivity
  • Transition Temperature
  • Transitions

Fields of Study

  • Physics

Readers

  • Combustion science or combustion engineering.