LASER RAMAN SCATTERING STUDIES OF CRYSTALS

Abstract

Temperature dependent Raman spectroscopy of quartz has revealed the existence of a new optical lattice vibration mode which appears to play a fundamental role in the alpha-beta phase transition. Continued temperature dependent Raman measurements of Strontium Titanate have also disclosed a new 'moving' component in the spectrum. Additional measurements have also shown that the three sharp Raman lines which are present at all temperatures below the 110 degrees K cubic to tetragonal transition probably arise from local breaking of the translational symmetry by inhomogeneous strain within the domain walls. Intensity vs. temperature measurements of the strong component at 78 reciprocal cm (room temperature value) have failed to confirm our earlier conclusion that part of the room temperature Raman spectrum of Strontium Titanate is of first order. Preliminary Raman measurements have been performed on KDP, and have failed to produce conclusive evidence for an anticipated 'soft' mode which was predicted by Cochran.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Aug 01, 1967
Accession Number
AD0658342

Entities

People

  • Herman Z. Cummins

Organizations

  • Johns Hopkins University

Tags

Communities of Interest

  • Human Systems

DTIC Thesaurus Topics

  • Argon Lasers
  • Beta Testing
  • Brillouin Scattering
  • Crystal Lattice Vibrations
  • Crystal Lattices
  • Frequency
  • Lasers
  • Measurement
  • Phase Transformations
  • Physics
  • Physics Laboratories
  • Raman Scattering
  • Raman Spectra
  • Raman Spectroscopy
  • Scattering
  • Spectra
  • Transition Temperature

Fields of Study

  • Physics

Readers

  • Materials Science and Engineering.
  • Optical Physics and Photonics.
  • Regression Analysis.

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers
  • Directed Energy - Pulsed-Laser Deposition