CARBIDE SYNTHESIS BY METAL EXPLOSIONS IN ACETYLENE

Abstract

Thermally stable metal carbides can be synthesized readily by electrical explosion of metals into acetylene. Reasonably high degrees of purity can be obtained under appropriate reaction conditions. An important factor governing the purity of the carbide product is the necessity for dilution of the acetylene reactant with an inert gas; this minimizes the rate of self-pyrolysis of acetylene to graphite and hydrogen. It was shown that explosive vaporization of the metal is not necessary for carbide formation since liquid droplets of the metal react readily with gaseous species derived from acetylene; thus explosive melting suffices. Using this technique, LaC2, TiC, ZrC, NbC, Nb2C, Ta2C, MoC, Mo2C, and W2C were prepared from the respective metals. Of the metals studied, only cobalt failed to form a carbide. Factors involved in the synthesis of specific carbides when the metal forms more than one stable carbide are discussed.

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Document Details

Document Type
Technical Report
Publication Date
Sep 01, 1967
Accession Number
AD0662580

Entities

People

  • Bernard Siegel
  • Eileen Cook

Organizations

  • The Aerospace Corporation

Tags

Communities of Interest

  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Acetylenes
  • Air Force
  • Alkynes
  • Ceramic Materials
  • Diffraction
  • Dilution
  • Electric Power
  • Energy Levels
  • Exothermic Reactions
  • Explosions
  • Graphitic Materials
  • Hydrocarbons
  • Metals
  • Pyrolysis
  • Titanium
  • Transition Metals
  • X-Ray Diffraction

Fields of Study

  • Chemistry

Readers

  • Combustion science or combustion engineering.
  • Powder metallurgy of Titanium alloys.