NONLINEAR OPTICAL SUSCEPTIBILITIES IN GROUP IV AND III-V SEMICONDUCTORS.
Abstract
The contribution of the valence electrons to the nonlinear optical susceptibilities may be estimated on the basis of simple telrahedral bonding orbitals. The coefficient for second harmonic generation in III-V compounds is in satisfactory agreement with the theoretical estimate. The same model contributes to the third-order nonlinearity, which describes scattering processes between four light waves. Again reasonable agreement is obtained with data for combination frequency generation in Si and Ge. The much larger effects in n-type InAs and InSb are due to conduction electrons. Their contribution has been calculated exactly if Kane's theory for the band structure is used. The contribution of the valence electrons is, however, not negligible and is equal to the contribution of 10 to the 16th power electrons/cc in InSb. (Author)
Document Details
- Document Type
- Technical Report
- Publication Date
- Jan 01, 1968
- Accession Number
- AD0665983
Entities
People
- Nicolaas Bloembergen
- Sudhanshu S. Jha
Organizations
- Harvard University