PHOTOREACTIONS OF REVERSIBLE BLEACHING OF DYES ADSORBED ON GLASS CAPILLARIES

Abstract

Absorbed methylene blue on microporous glass shows initially reversible bleaching under irradiation and regeneration with molecular oxygen in the presence of organic and inorganic bases. During the irradiation as a result of heating by the light, part of the dye monomer is converted to dimer which is not reversibly bleached. Photobleaching of the adsorbed dye occurs at low temperature (-180, -70 deg C) significantly more weakly than at room temperature. Capillary condensed oxygen at low temperature has almost no regenerating effect on the leucoform of the dye. Traces of iron present in the microporous glass do not influence the bleaching of adsorbed methylene blue, and the artificial introduction of iron facilitates not the bleaching process, but only the dimerisation of the dye under the action of light. The reversible photobleaching and regeneration of adsorbed dibenzypyrene-quinone on microporous glass in the presence of organic bases was observed. Additional experiments show the part played by surface OH groups on the porous glass and other adsorbents in the photoreduction of methylene blue.

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Document Details

Document Type
Technical Report
Publication Date
Jul 01, 1968
Accession Number
AD0682883

Entities

People

  • A. V. Karyakin

Organizations

  • United States Army Biological Warfare Laboratories

Tags

Communities of Interest

  • Air Platforms
  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Absorption
  • Absorption Spectra
  • Adsorbates
  • Adsorbents
  • Aqueous Solutions
  • Dyes
  • Glass
  • Hydrogen
  • Infrared Radiation
  • Low Temperature
  • Measurement
  • Methylene Blue
  • Methylenes
  • Redox Indicators
  • Silica Gels
  • Spectra
  • Water

Readers

  • Chemistry (specifically Chemical Fluorescence)
  • Surface Coatings Technology.