NEW SYNTHESES OF POLYBENZIMIDAZOLES,

Abstract

Polybenzimidazoles were synthesized from adipamide dihydrochloride, diethyl diiminoadipate dihydrochloride and 3,3' -diaminiobenzidine, and also from adiponitrile and 3,3' -diaminobenzidine tetrahydrochloride both in melt and in N-methylphrolidinone solution. The melting temperatures and the solubilities of poly prepared by these methods approached those of polybenzimidazoles of a similar structure prepared from diphenyl adipate and 3,3' -diamino-benzidine. The polymers are light-brown powders soluble in sulfuric and formic acids, dimethylformamide, dimethylsulfoxide, dimethylacetamide, and other solvents. The reduced viscosity of 0.5 percent solution of the polymers in formic acid at 25 degrees C was 0.5 dl/g. The structure of the polymer was confirmed by IR-spectroscopy and elemental analysis. (Author)

Document Details

Document Type
Technical Report
Publication Date
Jun 09, 1969
Accession Number
AD0691653

Entities

People

  • S. V. Vinogradova
  • V. A. Pankratov
  • V. V. Korshak

Organizations

  • National Air and Space Intelligence Center

Tags

DTIC Thesaurus Topics

  • Formic Acid
  • Polybenzimidazole
  • Polymers
  • Rigid Rod Polymers
  • Solubility
  • Solvents
  • Specialty Uses Of Chemicals
  • Spectroscopy
  • Viscosity

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry
  • Polymer Science and Engineering.
  • Polymer Science and Technology