DISCHARGE MECHANISM OF THE V2O5 ELECTRODE.

Abstract

The behavior of V2O5 single crystals, grown from the melt, during cathodic polarization and recovery, was investigated. The dependence of potential upon pH showed that the only plausible reduction product was a solid oxide or oxyhydroxide, polarization being due to the formation of a solid solution. In the pH range 2.0 - 5.5, the curve of electrode potential vs. time during both polarization and recovery was accurately predicted by an equation, already applied to MnO2, derived from the assumption that the product is removed from the surface by diffusion into the electrode. Using tritium as a tracer, it was shown that hydrogen is incorporated in the electrode during discharge at pH 4.7. The activation energy for diffusion was found to be 6.7 kcal/mole, which is consistent with bipolar diffusion of protons and electrons. (Author)

Document Details

Document Type
Technical Report
Publication Date
Aug 30, 1969
Accession Number
AD0693308

Entities

People

  • Allen B. Scott
  • Kenneth R. Newby

Organizations

  • Oregon State University

Tags

DTIC Thesaurus Topics

  • Crystals
  • Diffusion
  • Electrodes
  • Electrons
  • Energy
  • Equations
  • Heat Of Activation
  • Hydrogen
  • Polarization
  • Recovery
  • Single Crystals
  • Solid Solutions

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.
  • Plasma Physics.
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.

Technology Areas

  • Microelectronics