THE ROLE OF PASSIVE FILM GROWTH KINETICS AND PROPERTIES IN STRESS CORROSION SUSCEPTIBILITY

Abstract

The role of passivation kinetics, film ductility, and tarnish film formation in stress corrosion cracking were each examined in the following studies: (1) Ellipsometry measurements of film growth kinetics on iron have been made for two anions whose solution cause stress cracking of steel (nitrate and hydroxide) and two that do not (chloride and nitrite). (2) A technique has been developed to measure film ductility directly. This technique couples an ellipsometer with a tensile machine. Thin films on Ta show a ductility of 3-4% in the presence and absence of F(-), an ion thought to decrease ductility. (3) Pure copper forms tarnish films in cupric acetate and sulfate solutions. It is susceptible to stress corrosion cracking in cupric acetate solution. In the absence of stress, oxide forms all over the copper surface, while stress concentrates oxide formation at the grain boundaries. These experiments point ot a brittle-film rupture mechanism of stress cracking.

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Document Details

Document Type
Technical Report
Publication Date
Feb 28, 1970
Accession Number
AD0704882

Entities

People

  • Edward Escalante
  • Jerome Kruger
  • John Ambrose

Organizations

  • National Institute of Standards and Technology

Tags

DTIC Thesaurus Topics

  • Buffers (Chemistry)
  • Carbon Steels
  • Copper
  • Crystal Structure
  • Ductility
  • Films
  • Grain Boundaries
  • Hydroxides
  • Materials
  • Mechanical Properties
  • Metals
  • Rate Of Formation
  • Sodium Compounds
  • Stress Corrosion
  • Stress Corrosion Cracking
  • Stress Cracking
  • Thin Films

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies
  • Materials Science (Mechanical Engineering).
  • Thin Film Deposition Science.