A MOLECULAR ORBITAL INTERPRETATION OF THE SOFT X-RAY L(11,111) EMISSION AND ABSORPTION SPECTRA FROM SOME TITANIUM AND VANADIUM COMPOUNDS.

Abstract

A molecular-orbital energy-level diagram is constructed and used to interpret the metal-ion L(11,111) X-ray emission and absorption spectra from the oxides, nitrides, carbides, and borides of titanium and vanadium. It is shown that the MO model provides a more accurate description of the experimental results than did the ionic model and crossover transition theory. Specific electronic transitions are assigned to spectral components. Anomalous emission peaks which fall on the low energy side of the main L(111) band are found to originate in molecular orbitals which are primarily associated with ligand 2p and 2s levels. (Author)

Document Details

Document Type
Technical Report
Publication Date
Aug 01, 1970
Accession Number
AD0713100

Entities

People

  • David W. Fischer

Organizations

  • Air Force Research Laboratory

Tags

DTIC Thesaurus Topics

  • Absorption
  • Absorption Spectra
  • Emission
  • Energy Levels
  • Metals
  • Soft X Rays
  • Spectra
  • Titanium
  • Transitions
  • Vanadium
  • Vanadium Compounds
  • X Rays

Fields of Study

  • Physics

Readers

  • Quantum Chemistry
  • Spectroscopy.
  • Surface Engineering/Surface Coating Technology.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene
  • Space