SEARCH FOR A FOUR-MICRON MOLECULAR LASER.

Abstract

Experiments have been conducted in an effort to achieve continuous laser action in HCN, which has a vibrational transition at 3.86 microns, a wavelength which falls well within the atmospheric window just below 4 microns. Indirect excitation of the upper level (the C-H stretching fundamental) was accomplished by collisions with vibrationally excited hydrogen, deuterium, and nitrogen, without apparent decomposition of the HCN, which is known to suffer extensive decomposition when exposed to an electric discharge. The upper level (001) was identified by infrared emission spectroscopy, and its concentration was estimated to be several per cent at a pressure of 0.05 torr of HCN and 1 torr of discharge-excited H2. No oscillations were observed with HCN excited by H2 or N2 in a 1-meter flowing laser system even when dry-ice cooling was used to reduce the population of the lower (010) level, which is the bending fundamental. (Author)

Document Details

Document Type
Technical Report
Publication Date
Sep 01, 1970
Accession Number
AD0713193

Entities

People

  • John M. Flournoy

Tags

DTIC Thesaurus Topics

  • Atmospheric Windows
  • Collisions
  • Decomposition
  • Deuterium
  • Electric Discharges
  • Elements
  • Emission
  • Emission Spectroscopy
  • Excitation
  • Hydrogen
  • Laser Applications
  • Laser Spectroscopy
  • Lasers
  • Molecular Lasers
  • Nitrogen
  • Nonmetals
  • Spectroscopy

Fields of Study

  • Physics

Readers

  • Atmospheric Remote Sensing.
  • Molecular Photonics/Laser Physics

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers