Optical Spectrum of Triply Ionized Erbium in Calcium Tungstate,

Abstract

The energy levels of the quadruplet I ground term of Er(3+) in single crystals of CaWO4 were established by absorption and fluorescence spectra measurements. The measurements were made using crystals at temperatures of 2, 20, and 85K. The energy level scheme allows an interpretation of the 1.612-micron four-level CaWO4:Er(3+) laser transition and shows the terminal energy level of this transition to be 318/cm above the ground state rather than 375/cm as reported by Kiss and Duncan. An effective Hamiltonian of the form suggested by Karayianis was diagonalized in a basis of Russell-Saunders wave functions to obtain the calculated energy levels and wave functions for the entire ground term of Er(3+). The calculation takes into account the complete J-mixing of the states within the ground term and is equivalent to determining the effects of the spin-orbit interaction to better than second order. (Author)

Document Details

Document Type
Technical Report
Publication Date
Jun 01, 1970
Accession Number
AD0715008

Entities

People

  • Donald E. Wortman

Organizations

  • Harry Diamond Laboratories

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Crystals
  • Energy Levels
  • Ground State
  • Measurement
  • Quantum Properties
  • Single Crystals
  • Spectra
  • Spin-Orbit Interaction
  • Transitions
  • Wave Functions

Fields of Study

  • Physics

Readers

  • Materials Science and Engineering.
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers
  • Microelectronics
  • Space