Thermodynamics of Alloys
Abstract
Tin solution calorimetry has been used to measure the heats of formation of selected face-centered cubic palladium-rich solid solutions of the palladium-silver-tin system. The results show that alloys of constant electron concentration are characterised by heats of formation which vary almost exactly linearly between the values for the terminal binary alloys. The results are discussed in relation to the possible contributions associated with electronic energy and ion-ion interaction effects. Lattice parameters of the alloys have been measured and a linear variation of these is also observed. The technique based on the precipitation of an alloy phase from liquid tin has been used for the study of the aluminides Pt2Al3(Ni2Al3-type), RhAl (CsCl-type) and NiAl (CsCl-type), while normal solution calorimetry has been used to investigate the compound PdGa (FeSi-type). Values obtained for the heats of formation were found. These and previously determined heats of formation of related compounds are compared and trends and influences in the heats of formation of transition metal aluminides and palladium - Group IIIB compounds are discussed.
Document Details
- Document Type
- Technical Report
- Publication Date
- Jan 01, 1971
- Accession Number
- AD0722799
Entities
People
- A. W. Bryant
- D. T. Underhill
- John N. Pratt
Organizations
- University of Birmingham