Stimulated Light Scattering in Binary Gas Mixtures

Abstract

The theory of stimulated light scattering from a binary gas mixture was developed. It considers the coupling of a laser wave and a scattered light wave with the collective modes of the mixture. It was found that in a binary gas mixture in which the different types of molecules have a large difference in mass and polarizability, it is possible to generate stimulated scattering from local fluctuations in the concentration. The shift in frequency between the laser and backward scattered wave was observed systematically as a function of helium concentration from 0 to 90% in mixtures of He and SF6 in which the partial pressure of SF6 was 5 atm., and in mixtures of He and Xe in which the partial pressure of Xe was 8 atm. In both cases, for helium concentration less than 60% the frequency shift of the backscattered light is characteristic of stimulated Brillouin scattering in the mixture. As the helium concentration increases above 60%, the frequency shift decreases and rapidly approaches the small values which are characteristic of stimulated concentration scattering. The experimental observations are in good agreement with theoretical predictions.

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Document Details

Document Type
Technical Report
Publication Date
Jun 01, 1971
Accession Number
AD0726469

Entities

People

  • H. Lowdermilk
  • Nicolaas Bloembergen

Organizations

  • Harvard University

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Brillouin Scattering
  • Diffraction
  • Electromagnetic Fields
  • Electromagnetic Scattering
  • Fluid Dynamics
  • Frequency Shift
  • Ideal Gas Law
  • Laser Beams
  • Light Scattering
  • Measurement
  • Optics
  • Optomechanics
  • Partial Pressure
  • Refractive Index
  • Standing Waves
  • Thermal Conductivity
  • Thermodynamics

Fields of Study

  • Physics

Readers

  • Molecular Photonics/Laser Physics
  • Optical Physics and Photonics.

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers