The Quenching of O(singlet D) by N2 and Related Reactions
Abstract
As an extension of earlier work on the quenching of electronically excited alkali metal atoms by N2 and CO, which uses a model of curve crossing involving an ionic intermediate state, here the authors treat the quenching of O(singlet D) by N2, a process which proceeds by curve crossing of covalent states. The model is also applied to the vibrational relaxation of N2 in collision with O(triplet P) atoms and to the unimolecular decomposition of N2O. The order of magnitude of the rate constants for all 3 processes can be explained by the present model, using the same value of the electronic coupling potential for the curve-crossing process.
Document Details
- Document Type
- Technical Report
- Publication Date
- Dec 01, 1971
- Accession Number
- AD0736700
Entities
People
- Edward R. Fisher
- Ernest Bauer
Organizations
- Institute for Defense Analyses