About the Forming of the Structure of Pyrolytic Carbonic Fibers,

Abstract

Rayon fibers are oxidized with N oxides to poly(anhydrouronic acids) which are converted to the Al salts. The pyrolysis of fibers containing 11.5 percent COOH groups is carried out in a vacuum up to 850 degrees by raising the temperature at a 4 degrees minimum rate. Higher yields of carbon fibers with higher rigidity are obtained from rayons containing higher proportion of the COOH groups. Oxidation to 50 percent give optimal properties and yields. The pyrolysis temperature strength relation shows a minimum strength at 200 degrees and a substantial increase in the strength at 800- 850 degrees. Gas adsorption and the IR study demonstrate that the carbon fibers represent a highly packed structure of oriented molecules. Preoxidation and Al-salts enhance the formation of oriented structures. Slower rate of temperature raise during the pyrolysis or longer heating at 800 degrees, as well as drawing the fibers during the pyrolysis, increase the mechanical strength of the carbon fibers. (Author, modified-PL)

Document Details

Document Type
Technical Report
Publication Date
Nov 12, 1971
Accession Number
AD0739284

Entities

People

  • I. N. Ermolenko
  • R. N. Sviridova

Organizations

  • National Air and Space Intelligence Center

Tags

DTIC Thesaurus Topics

  • Adsorption
  • Carbon Fibers
  • Chemical Compounds
  • Chemical Reactions
  • Fibers
  • Molecules
  • Ores
  • Oxidation
  • Oxides
  • Oxygen Compounds
  • Pyrolysis
  • Rigidity
  • Rocks And Deposits

Readers

  • Optical Physics and Photonics.
  • Polymer Science and Engineering.
  • Thin Film Deposition Science.