Bipotentiometry in Organic Redox Systems. 1. Oxidation of Aromatic Compounds in Trifluoroacetic Acid

Abstract

Bipotentiometric titrations of various polynuclear aromatic hydrocarbons, benzenes substituted with electron-donating groups, and pi- excessive heteroaromatics in trifluoroacetic acid - dichloromethane with lead (IV) or cobalt (III) acetate solution resulted in novel titration curves. Each reagent increment usually resulted in the formation of a potential 'saw tooth,' indicating formation and decay of reversible redox couples; the final titration curves had one or more potential minima regions before the end-point. In almost all instances the titration curve for a given aromatic compound is characteristic, somewhat in the manner of a spectrophotometric curve.

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Document Details

Document Type
Technical Report
Publication Date
Jun 22, 1970
Accession Number
AD0741025

Entities

People

  • Harvey W. Yurow
  • Samuel Sass

Tags

DTIC Thesaurus Topics

  • Aromatic Compounds
  • Aromatic Hydrocarbons
  • Chemical Laboratories
  • Chemical Synthesis
  • Chemistry
  • Cyclic Hydrocarbons
  • Electron Transfer
  • Electrons
  • Hydrocarbons
  • Maryland
  • Materials
  • New York
  • Organic Chemistry
  • Oxidation
  • Reversible
  • Spin Resonance
  • Titration

Fields of Study

  • Chemistry

Readers

  • Approximation Theory.
  • Electrochemical Surface Science
  • Organic Chemistry

Technology Areas

  • Microelectronics