The Thermal and Catalytic Decomposition of Methylhydrazines

Abstract

The thermal decomposition of methylhydrazine (MMH), 1,1- dimethylhydrazine (UDMH) and trimethylhydrazine (TMH) using a time of flight mass spectrometer is discussed and the catalytic decomposition of MMH and UDMH over heated Shell 405, a spontaneous hydrazine decomposition catalyst, is also reported. Both the catalyzed and uncatalyzed experiments were conducted using a heated quartz chamber directly preceding the leak to the mass spectrometer. The temperature range was from ambient to an upper limit of 1000C. The main products of the thermal degradation of the methyl derivatives of hydrazine are hydrogen cyanide (HCN), nitrogen (N2), and ammonia (NH3); in the catalytic decomposition the main products are N2 and H2, as the NH3 originally formed is decomposed by Shell 405 to yield N2 and H2.

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Document Details

Document Type
Technical Report
Publication Date
Jul 01, 1972
Accession Number
AD0749262

Entities

People

  • Henry A. Nappier
  • James A. Murfree Jr.
  • John Phillips
  • Pasquale Martignoni
  • William A. Duncan

Tags

Communities of Interest

  • Weapons Technologies

DTIC Thesaurus Topics

  • Catalysts
  • Chemical Reactions
  • Chemistry
  • Decomposition
  • Degradation
  • Dimethylhydrazines
  • Dissociation
  • Elements
  • Hydrazine Derivatives
  • Hydrazines
  • Hydrogen
  • Ionization
  • Mass Spectra
  • Mass Spectrometers
  • Pyrolysis
  • Spectra
  • Spectrometers

Readers

  • Combustion science or combustion engineering.
  • Organic Chemistry
  • Underwater engineering and Marine Technology.