Thermal Degradation of High Temperature Polymers and Composites

Abstract

A study was performed to examine the thermal degradation process and char forming characteristics of a number of polyquinoxaline polymers. The techniques used were primarily of thermogravimetry, differential thermal analysis, and mass spectrometry. Constant heating rate and isothermal degradation experiments were carried out in vacuum, and to some extent, in air; the isothermal degradation rates were used to obtain an approximate activation energy for the degradation process. The quinoxaline-based polymers showed improved thermal stability and greater carbon yields compared to conventional polymers. Thermal degradation occurred in three discrete steps. Generalized degradation mechanisms that have been derived for these polymers from combined mass spectrometry and residue analysis results are described.

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Document Details

Document Type
Technical Report
Publication Date
Jun 23, 1972
Accession Number
AD0750396

Entities

People

  • C. A. Gaulin
  • W. H. Pfeifer

Organizations

  • Battelle Memorial Institute

Tags

Communities of Interest

  • Advanced Electronics
  • C4I
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Ablative Materials
  • Carbon Monoxide
  • Chemical Synthesis
  • Chemistry
  • Composite Materials
  • Dielectric Gases
  • Ethers
  • Heat Shields
  • High Temperature
  • Mass Spectrometry
  • Measurement
  • Organic Chemistry
  • Phenyl Ether
  • Plastic Explosives
  • Spectrometry
  • Thermal Analysis
  • Three Dimensional

Readers

  • Calculus or Mathematical Analysis
  • Electrochemical Engineering/ Fuel Cell Technologies
  • Polymer Science and Engineering.