Measurement of Vibrational Temperature of CO and N2 Using the He(2 triplet S) Penning Ionization Technique.

Abstract

The vibrational temperatures of N2 and CO in binary gas mixture and in the VV quasi-equilibrium regime of high vibrational temperature and low kinetic temperature were measured in a flow tube apparatus. The Penning ionization with He(2 triplet S) technique was used to determine the vibrational temperatures of both gases. The Treanor-Teare expression relating vibrational temperatures relating vibrational temperatures for such conditions was verified. The formulation of the Penning ionization technique for CO allowed the CO rotational energy and the kinetic energy of relative motion between CO and He to play a role in the normally nonenergetically allowed CO(X, 0) to CO(+)(B,1) excitation reaction. The unexpected result of a collisional quenching rate that is smaller for CO(+)(B,1) than for CO(+)(B,0) was also observed. (Author)

Document Details

Document Type
Technical Report
Publication Date
Sep 25, 1972
Accession Number
AD0751466

Entities

People

  • Stephen J. Young

Organizations

  • The Aerospace Corporation

Tags

DTIC Thesaurus Topics

  • Chemical Reaction Properties
  • Energy
  • Excitation
  • Ionization
  • Kinetic Energy
  • Measurement
  • Quenching
  • Relative Motion

Fields of Study

  • Physics

Readers

  • Military and Counterinsurgency Studies.
  • Molecular Photonics/Laser Physics