Pyrolysis-Molecular Weight Chromatography of Polymers.

Abstract

A pyrolyzer with programming capability has been coupled in series with a thermal conductivity cell and a mass chromatograph. The thermal conductivity cell gives the flexibility for selective trapping of decomposition products, and also provides data that are complementary to thermogravimetric and differential thermal analyses. The mass chromatograph is composed of two gas chromatographs that are run parallel from a common injection port. Each chromatograph uses a different carrier gas, and is equipped with a gas density balance detector. The instrument simplifies identification of mixtures of unknowns in directly providing molecular weights, absolute quantities and gas chromatographic retention times of the constituents. In this respect, the present system is analogous to pyrolysis-gas chromatography-mass spectrometry. Discussion of the technique and its application to the investigation of the thermal degradation of low density polyethylene are presented. (Author)

Document Details

Document Type
Technical Report
Publication Date
Apr 01, 1973
Accession Number
AD0758711

Entities

People

  • E. Kiran
  • J. K. Gillham

Organizations

  • Princeton University

Tags

DTIC Thesaurus Topics

  • Chromatographs
  • Chromatography
  • Conductivity
  • Detectors
  • Differential Thermal Analysis
  • Gas Chromatography
  • Low Density
  • Mass Spectrometry
  • Materials
  • Molecular Weight
  • Pyrolysis
  • Spectrometry
  • Spectroscopy
  • Thermal Analysis
  • Thermal Conductivity

Readers

  • Analytical Chemistry
  • Polymer Science and Engineering.
  • Thermal Physics or Thermal Science.