Kinetics of Hydrazine Decomposition on Iridium and Alumina Supported Iridium Catalysts

Abstract

The kinetics of heterogeneous hydrazine decomposition were determined over the temperature range of 460 to 700K for a polycrystalline iridium surface, and the temperature range of 350 to 450K for an alumina supported iridium catalyst. A change in reaction mechanism and/or number of active catalytic sites was observed at approximately 450K for each catalyst. This is attributed to the irreversible, dissociate adsorption of hydrazine on a significant number of catalytic sites below 450K. Catalyst attrition mechanisms in monopropellant hydrazine engines are discussed in the light of this kinetic behavior. Recommendations are made concerning further elucidation of basic processes taking place in monopropellant engine cold starts.

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Document Details

Document Type
Technical Report
Publication Date
Aug 01, 1973
Accession Number
AD0766698

Entities

People

  • Owen I. Smith
  • Wayne C. Solomon

Organizations

  • Air Force Research Laboratory

Tags

Communities of Interest

  • Air Platforms
  • Weapons Technologies

DTIC Thesaurus Topics

  • Air Force
  • Aluminum Oxides
  • Chemical Reactions
  • Crystals
  • Detection
  • Electron Energy
  • Electrons
  • Energy
  • Heat Of Activation
  • Isotherms
  • Low Temperature
  • Measurement
  • Metals
  • Plastic Explosives
  • Propellants
  • Rocket Propulsion
  • Vapor Pressure

Fields of Study

  • Chemistry

Readers

  • Aerospace Propulsion Engineering.
  • Organic Chemistry
  • Thin Film Deposition Science.