Preparation and Single Crystal Growth of LiYF4 Laser Materials.

Abstract

The report describes techniques for preparation of high purity fluorides suitable for laser crystal hosts. Growth methods for LiYF4 were also developed using a constant flow of HF. The YF3 and rare earth fluorides are prepared from 5 or 6-9's polycrystalline oxides. A special platinum reactor was designed to convert oxides to fluorides via an HF reaction. Trifluorides were prepared at 800-900C and melted under HF at 1050-1200C. This prevented formation of oxide and oxyfluoride impurities in the melt. Growth of LiYF4 was accomplished in a resistively heated platinum apparatus and crucible using a modified Czochralski method. Growth occurred under a fixed pressure of HF. Preliminary results gave crystals of high optical quality, free of OH(-), scattering sites, and low impurity level. The procedures should be applicable to other YLF materials in volume production. (Author)

Document Details

Document Type
Technical Report
Publication Date
Feb 01, 1974
Accession Number
AD0775211

Entities

People

  • Durand R. Kinloch
  • Richard C. Puttbach
  • Robert Uhrin
  • Roger F. Belt

Tags

DTIC Thesaurus Topics

  • Crucibles
  • Crystal Growth
  • Crystals
  • Fluorides
  • Impurities
  • Laser Materials
  • Materials
  • Optical Materials
  • Platinum
  • Polycrystals
  • Production
  • Scattering
  • Single Crystals

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.

Technology Areas

  • Directed Energy