FABRICATION OF ULTRATHIN SOLID ELECTROLYTE BATTERIES.

Abstract

Further experiments were conducted with thin-film silver iodide, silver bromide, and KAg4I5 electrolyte cells. Problems of current leakage were eliminated by using quartz substrates. Silver iodide electrolyte cells were prepared in a nonoverlapping format on quartz. Cells charged to 0.485 V exhibited excellent voltage stability and shelf life of over two months. It was possible to fabricate Pt/AgI/Ag cells approx. 5 microns thick in an overlapping format, and by maintaining the voltage of the cell in vacuum during fabrication, we ensured considerable reproducibility of the fabrication method. Nonoverlapping symmetrical Ag/AgI/Ag cells exhibit strain gauge characteristics and may be used as stress-sensing devices. Silver bromide electrolyte cells have shelf life, and overlapping Au/AgBr/Ag cells 8-10 microns thick were prepared and tested successfully. A mixed salt electrolyte (KAg4I5) was prepared and successfully evaporated, and the charge-discharge characteristics of Pt/KAg4I5/Ag nonoverlapping cells were studied. Thin-film cells exhibited an increase in dc internal resistance with aging which may have been caused by the formation of a Pt or Au halide layer, voids in the Ag electrode-electrolyte interface, or actual degradation of the electrolytes. Evaporated silver films showed a tendency to disappear from silver halide electrolyte surfaces possibly because of neutral iodine present in the evaporated electrolyte. (Author)

Document Details

Document Type
Technical Report
Publication Date
Oct 01, 1967
Accession Number
AD0824398

Entities

People

  • J. Clune
  • J. I. Masters
  • P. Vouros

Tags

DTIC Thesaurus Topics

  • Degradation
  • Electrodes
  • Electrolytes
  • Fabrication
  • Films
  • Gages
  • Halides
  • Reproducibility
  • Resistance
  • Shelf Life
  • Silver Halides
  • Strain Gages
  • Thin Films

Fields of Study

  • Materials science

Readers

  • Battery Technology and Engineering
  • Electrochemical Engineering/ Fuel Cell Technologies
  • Thin Film Deposition Science.