MICROSCOPIC THEORY OF FERROELECTRICITY.
Abstract
A detailed formulation is given to the supposition that a polarized phase in ionic dielectrics can arise from the vibronic instability mechanism (Jahn-Teller effect) due to the valence electrons. The thermodynamical consequences of this hypothesis are worked out for BaTiO3. The contribution of the vibronic coupling to the temperature dependence of the soft mode in BaTiO3 is calculated. We use a frequency renormalization method to derive the effect of the soft mode on other long wavelength modes near the transitions. Last, the behavior of the optical vibrational frequencies in a finite-sized (or domain-structured) specimen is studied. (Author)
Document Details
- Document Type
- Technical Report
- Publication Date
- Nov 01, 1967
- Accession Number
- AD0825499
Entities
People
- Haim Yatom
- Raphael Ruppin
- Robert Englman
Organizations
- Israel Atomic Energy Commission