Electrode-Electrolyte Interactions Magnesium Anodes: meta-Dinitrobenzene Cathodes

Abstract

The electrochemical dissolution of magnesium (AZ-21) and the h.e.r. on magnesium (AZ-21) in magnesium perchlorate, sodium perchlorate and a mixed electrolyte of sodium and magnesium perchlorate has been investigated. In the sodium perchlorate electrolyte, 0.4M to 4.0M, the Tafel Slope of the h.e.r. was unaffected by the direction of the potential sweep. In the magnesium perchlorate electrolyte, 0.2M to 2.0M, the Tafel Slope of the h.e.r. changes with direction of the potential sweep. The anodic Tafel Slopes in the pure electrolytes was 50 mv and 30 mv in the mixed electrolytes. The rate of magnesium dissolution in the magnesium perchlorate was about an order of magnitude faster than that in the sodium perchlorate electrolyte. On the other hand the corrosion current density of magnesium in the magnesium perchlorate was three orders of magnitude greater than in the sodium perchlorate electrolyte. Corrosion rates of magnesium in magnesium perchlorate and magnesium perchlorate saturated with magnesium hydroxide was also investigated. It was found that addition of the hydroxide reduced the corrosion rate by about 50%. It was also determined that magnesium did not exhibit the Negative Difference Affect.

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Document Details

Document Type
Technical Report
Publication Date
Dec 01, 1969
Accession Number
AD0865587

Entities

People

  • Akim Adubifa
  • Gerald Smaldone
  • Gideon Stern
  • Leonard L. Wikstrom

Organizations

  • New York University

Tags

Communities of Interest

  • Ground and Sea Platforms

DTIC Thesaurus Topics

  • Acetic Acid
  • Alloys
  • Body Weight
  • Corrosion
  • Current Density
  • Efficiency
  • Electrochemical Cells
  • Electrochemical Reactions
  • Electrodes
  • Electrolytes
  • Hydroxides
  • Magnesium
  • Magnesium Alloys
  • Magnesium Hydroxide
  • New York
  • Perchlorates
  • Polarization

Fields of Study

  • Materials science

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies
  • Materials Science and Engineering.