Utilizing the Power of Nanostructures to Their Fullest Capability in Energetic Formulations

Abstract

The significantly enhanced energy release expected from energetic formulations containing nanostructured aluminum (Al) has never been realized due to sintering of the nano-Al just prior to the energy release step. This precludes achieving the faster energy release, more efficient combustion, and controllable explosive performance consistent with the introduction of nanostructured metallics to energetic formulations. This DRI project used complementary experimentation and theory to study the energy release mechanisms of decompositions of novel assemblies of gas generators containing nanoscale Al (conventional Al nanoparticles and Al nanoclusters) to overcome the sintering and/or oxide-formation issues. Experimentally, a previously published hypothesis for the mechanism leading to enhanced energy release from Al nanoparticles in the presence of a gas generator was disproven, and a new hypothesis was developed. Computer simulations demonstrated that an unexpected intermixing inhibits the effect of small-scale Al clusters passivated with a gas generator, introducing different hindrances to enhanced combustion.

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Document Details

Document Type
Technical Report
Publication Date
Feb 01, 2016
Accession Number
AD1004629

Entities

People

  • Eric S. Collins
  • Iskander G. Batyrev
  • Jennifer L Gottfried
  • Michael R. Zachariah
  • N. S. Weingarten

Organizations

  • United States Army Research Laboratory

Tags

Communities of Interest

  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Combustion
  • Energetic Materials
  • Equations Of State
  • Explosives
  • Insensitive Explosives
  • Materials
  • Materials Laboratories
  • Materials Processing
  • Materials Science
  • Materials Testing
  • Metallic Nanoparticles
  • Molecular Dynamics
  • Nanoparticles
  • Nanostructures

Fields of Study

  • Physics

Readers

  • Combustion science or combustion engineering.
  • Nanocomposite Materials Science
  • Systems Analysis and Design

Technology Areas

  • Biotechnology
  • Microelectronics