Development of Nanomedicines for Treatment of Posttraumatic Osteoarthritis

Abstract

For this project, N-(2-hydroxypropyl) methacrylamide (HPMA) copolymer conjugates (including dexamethasone and BMS-345541 conjugates) were synthesized and labeled with near-infrared dye IRDye CW 800, Alexa Fluor 488 or Alexa Fluor 647. Mice with surgical destabilization of the medial meniscus (DMM) were established as an osteoarthritis model for our evaluation. P-IRDye and P-Alexa were given to the DMM mice via intraarticular injection. Optical imaging demonstrated that the DMM joints retained the injected P-IRDye. Fluorescence microscopy studies, in line with the in vivo imaging results, confirmed that P-Alexa was retained within the joint space and was primarily localized to synovial lining cells and articular chondrocytes. To further confirm the ability of chondrocytes to retain the copolymer conjugates, mouse femoral head explants were cultured in presence of P-Alexa. Imaging confirmed internalization of the conjugate by chondrocytes. Cell culture studies demonstrated that P-Alexa was sequestered within an endosomal/lysosomal compartment. Cell culture studies showed that P-BMS, a NF-B inhibitor copolymer conjugate, inhibited LPS induction of pro-inflammatory cytokine expression and provided sustained inhibition of osteoclast formation.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Mar 01, 2016
Accession Number
AD1008164

Entities

People

  • Dong Wang
  • P. E. Purdue
  • Steven R. Goldring

Organizations

  • University of Nebraska Omaha

Tags

DTIC Thesaurus Topics

  • Arthritis
  • Cartilage
  • Cells
  • Connective Tissue Cells
  • Copolymers
  • Culture Techniques
  • Cytokines
  • Data Analysis
  • Diseases And Disorders
  • Fluorescence
  • Joints (Anatomy)
  • Macrophages
  • Medical Personnel
  • Microscopy
  • Polymers
  • Tissues

Readers

  • Chemistry (specifically Chemical Fluorescence)
  • Immunology and Pathology
  • Neurotrauma and Rehabilitation Medicine.

Technology Areas

  • Biotechnology
  • Biotechnology - Cancer Biotech
  • Microelectronics
  • Space