Assessment of Metaborate Fusion for the Rapid Dissolution of Solid Samples: Suitability with the Northstar ARSIIe

Abstract

The original goal of this project was to develop a rapid dissolution methodology for solid environmental samples and a crude pre-concentration of actinides (uranium, plutonium, thorium, americum) following the dissolution process to enable compatibility with the Automated Radionuclide Separation System-Environmental (ARSIIe) from Northstar Engineered Technologies. It was later required by the client during a subsequent meeting (August 2012, Quebec City, Quebec, Canada) that strontium be included in the list of analytes for which the sample preparation methodology should be applicable. This project was accomplished by executing a rigorous research and development strategy for soil dissolution that focuses on field deployment, efficiency, and the resulting dissolution being compatible with radiochemical separation performed by the ARSIIe using compatible designed protocols (necessary for controls and reproducibility). It was required by the client that the method of dissolution be simple (field-deployable), reliable, complete, and contained in as small a volume as possible (10- to 20-mL target). In addition, up to 1 gram of solid environmental samples needed to be solubilized through a lithium metaborate fusion technique, using the M4 Fluxer unit from Corporation Scientifique Claisse.

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Document Details

Document Type
Technical Report
Publication Date
Jul 01, 2016
Accession Number
AD1017464

Entities

People

  • Annie Michaud
  • Dominic Lariviere

Tags

Communities of Interest

  • Advanced Electronics
  • Biomedical

DTIC Thesaurus Topics

  • Acids
  • Actinides
  • Air Force
  • Air Force Research Laboratories
  • Alkaline Earth Metals
  • Aqueous Solutions
  • Corporations
  • Hydroxides
  • Oxidation
  • Phosphoric Acids
  • Plutonium
  • Polyethylene Glycols
  • Polyethylenes
  • Resins
  • Silica Gels
  • Silicon Dioxide
  • Strontium

Readers

  • Analytical Chemistry
  • Distributed Systems and Data Platform Development
  • Materials Science and Engineering.