Quantification of Tetramethylenedisulfotetramine (TETS) in Various Food Matrices by Solid Phase Extraction Liquid ChromatographyIon Trap Mass Spectrometry

Abstract

Tetramethylenedisulfotetramine (TETS), commonly known as tetramine, is a highly neurotoxic rodenticide (the LD50, or lethal dose for 50 of test subjects, is 0.1 mg/kg). TETS has been used in hundreds of deliberate and accidental food poisoning events in China. In this report, we describe an extraction method for the quantitation of TETS as spiked into various food matrices, including fruit juices, egg, hot dog, chicken nuggets, turkey deli meat, and ground beef. Quantitation by liquid chromatographyion trap mass spectrometry was based upon selected reaction monitoring of mass-to-charge ratio (m/z) 347 268 and consecutive reaction monitoring of m/z 347268175. An ~5 mg TETS concentration was spiked into each food sample. The linear range of quantitation for TETS was 0.520 g/mL. Total recoveries (and percent relative standard deviations) for TETS in various food samples are reported.

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Document Details

Document Type
Technical Report
Publication Date
Apr 01, 2017
Accession Number
AD1032301

Entities

People

  • Li Kong
  • Sue Y. Bae

Organizations

  • Edgewood Chemical Biological Center

Tags

Communities of Interest

  • Counter WMD
  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Chemical Reactions
  • Chromatography
  • Electrospray Ionization
  • Food Poisoning
  • Gas Chromatography
  • Ion Traps
  • Lethal Dosage
  • Liquid Chromatography
  • Mass Spectra
  • Mass Spectrometry
  • Monitoring
  • Phase
  • Poisoning
  • Rodenticides
  • Solid Phases
  • Spectrometry
  • Standards

Fields of Study

  • Chemistry

Readers

  • Gender and Food Studies
  • Naval Engineering and Maritime Security
  • Oncology and Biomarker-Based Cancer Detection.