Probing Molecular Ions With Laser-Cooled Atomic Ions

Abstract

The overall theme of this project was to explore methods for using laser-cooled atomic ions to probe information about molecular ions. The initial goal was to focus on the atomic assisted spectroscopy of BH for direct laser-cooling of BH+. In the first year, the direct loading of BH+ remained elusive and the goals were changed to developing spectroscopy techniques for CaH+. These goals included sideband cooling of CaH+, resonance enhanced multiphoton dissociation spectroscopy of CaH+ in a Coulomb crystal, and quantum logic spectroscopy of CaH+. The first two goals have been completed and the third goal is in progress in our lab. We note that NIST Boulder has achieved quantum logic spectroscopy in CaH+ using the results obtained in our lab to design their experiment.

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Document Details

Document Type
Technical Report
Publication Date
Oct 11, 2017
Accession Number
AD1050677

Entities

People

  • Kenneth R. Brown

Organizations

  • Georgia Tech Research Corporation

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Ablation
  • Abstracts
  • Chemical Kinetics
  • Cooling
  • Dissociation
  • Femtosecond Lasers
  • Ground State
  • Laser Cooling
  • Lasers
  • Measurement
  • Molecular Spectroscopy
  • Sidebands
  • Spectra
  • Spectroscopy
  • Students
  • Theses
  • Transitions

Fields of Study

  • Physics

Readers

  • Molecular Photonics/Laser Physics
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.

Technology Areas

  • Directed Energy
  • Quantum Computing