Section II, A2, G-7.5 Metal-Organic Framework Materials for Force Protection

Abstract

(I) A Ce(IV)-based metal-organic framework (MOF) has been tested for the hydrolysis of a nerve agent simulant and the nerve agent, soman (GD) for the first time. Degradation half-lives of 8 min and 3 min were found for the simulant and nerve agent, respectively when using an N-ethylmorpholine buffer solution. A heterogeneous polyethyleneimine buffer was also used with the Ce-MOF catalyst and resulted in even faster hydrolysis of the simulant (t1/2 = 4.5 min). These results highlight the efficiency of Ce(IV)-based MOFs for hydrolysis of phosphate-ester based nerve agents.

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Document Details

Document Type
Technical Report
Publication Date
Apr 19, 2018
Accession Number
AD1054068

Entities

People

  • Joseph T. Hupp
  • Omar Farha

Organizations

  • Northwestern University

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Buffers (Chemistry)
  • Catalysis
  • Catalysts
  • Chemical Synthesis
  • Chemical Warfare
  • Chemical Warfare Agents
  • Chemistry
  • Composite Materials
  • Electron Microscopy
  • Films
  • Force Protection
  • Materials
  • Materials Science
  • Mustard Agents
  • Nerve Agents
  • Organophosphates
  • Oxygen

Readers

  • Nanocomposite Materials Science
  • Neurotoxicology
  • Parallel and Distributed Computing.