Observation of Vibrational Overtones by Single-Molecule Resonant Photodissociation

Abstract

Molecular ions can be held in a chain of laser-cooled atomic ions by sympathetic cooling. This system is ideal for performing high-precision molecular spectroscopy with applications in astrochemistry and fundamental physics. Here we show that this same system can be coupled with a broadband laser to discover new molecular transitions. We use three-ion chains of Ca and CaH to observe vibrational transitions via resonance-enhanced multiphoton dissociation detected by Ca fluorescence. On the basis of theoretical calculations, we assign the observed peaks to the transition from the ground vibrational state,n0 to n9 and 10. Our method allows us to track single-molecular events, and it can be extended to work with any molecule by using normal mode frequency shifts to detect the dissociation. This survey spectroscopy serves as a bridge to the precision spectroscopy required for molecular ion control.

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Document Details

Document Type
Technical Report
Publication Date
Jul 22, 2015
Accession Number
AD1058160

Entities

People

  • Gang Shu
  • Kenneth R. Brown
  • Ncamiso B. Khanyile

Organizations

  • Georgia Tech

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Base Pressure
  • Blackbody Radiation
  • Chemical Kinetics
  • Chemistry
  • Dissociation
  • Energy Levels
  • Frequency
  • Frequency Shift
  • Ground State
  • Infrared Lasers
  • Lasers
  • Mass Spectrometry
  • Measurement
  • Physical Chemistry
  • Spectra
  • Spectroscopy
  • Ultraviolet Lasers

Fields of Study

  • Physics

Readers

  • Explosive Engineering.
  • Molecular Photonics/Laser Physics
  • Positioning, Navigation, and Timing (PNT) Technology.

Technology Areas

  • Directed Energy