Ultrafast Relaxation of Hot Phonons in Graphene hBN Heterostructures

Abstract

Fast carrier cooling is important for high power graphene based devices. Strongly coupled optical phonons play a major role in the relaxation of photoexcited carriers in graphene. Heterostructures of graphene and hexagonal boron nitride (hBN) have shown exceptional mobility and high saturation current, which makes them ideal for applications, but the effect of the hBN substrate on carrier cooling mechanisms is not understood. We track the cooling of hot photo-excited carriers in graphene-hBN heterostructures using ultrafast pump-probe spectroscopy. We find that the carriers cool down four times faster in the case of graphene on hBN than on a silicon oxide substrate thus overcoming the hot phonon bottleneck that plagues cooling in graphene devices.

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Document Details

Document Type
Technical Report
Publication Date
May 08, 2017
Accession Number
AD1059580

Entities

People

  • Alexandra Brasington
  • Arvinder Sandhu
  • Brian J LeRoy
  • Dheeraj Golla

Tags

DTIC Thesaurus Topics

  • Carbon Nanotubes
  • Ceramic Materials
  • Charge Carriers
  • Chemical Vapor Deposition
  • Crystal Lattice Vibrations
  • Fullerenes
  • Graphene
  • Heat Capacity
  • Heat Transfer
  • Materials
  • Materials Laboratories
  • Materials Processing
  • Materials Science
  • Raman Spectroscopy
  • Semiconductors
  • Spectroscopy
  • Surface Plasmon Polaritons

Fields of Study

  • Physics

Readers

  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene