Gaps and pseudogaps in perovskite rare earth nickelates

Abstract

We report on tunneling measurements that reveal the evolution of the quasiparticle state density in two rare earth perovskite nickelates, NdNiO3 and LaNiO3, that are close to a bandwidth controlled metal to insulator transition. We measure the opening of a sharp gap of ~30 meV in NdNiO3 in its insulating ground state. LaNiO3, which remains a correlated metal at all practical temperatures, exhibits a pseudogap of the same order. The results point to both types of gaps arising from a common origin, namely, a quantum critical point associated with the T = 0 K metal-insulator transition. The results support theoretical models of the quantum phase transition in terms of spin and charge instabilities of an itinerant Fermi surface.

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Document Details

Document Type
Technical Report
Publication Date
Apr 23, 2015
Accession Number
AD1062213

Entities

People

  • Adam J. Hauser
  • Alex Kozhanov
  • Daniel G. Ouellette
  • Evgeny Mikheev
  • Jack Y. Zhang
  • James Kally
  • Junwoo Son
  • Leon Balents
  • Nelson E. Moreno
  • S. J. Allen
  • Susanne Stemmer

Organizations

  • University of California

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Band Structures
  • Bandwidth
  • Critical Temperature
  • Dielectrics
  • Electrons
  • Fermi Levels
  • Films
  • Ground State
  • Low Temperature
  • Materials
  • Metal-Insulator Transitions
  • Metals
  • Phase Transformations
  • Resistance
  • Transition Metals
  • Transition Temperature
  • Transitions

Fields of Study

  • Physics

Readers

  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.
  • Solar Photovoltaics and Thermoelectric Devices.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene
  • Quantum Computing