Environmental Fate of Remifentanil in Soil and Relevant Waters

Abstract

In this study, we assessed the stability and persistence of remifentanil in four water sources, buffered and unbuffered water, four different types of soil in contact with water containing 0.01 M CaCl2, and several soilwater environments. In unbuffered water samples, remifentanil appeared to degrade following first-order kinetics. A slightly acidic citrate buffer appeared to stabilize the remifentanil. Soil samples were spiked with a known amount of remifentanil in solution; the aqueous and solid (soil) layers were separated and extracted after contact times up to 11 weeks to track compound distribution and recovery. The analyte was detected in several of the aqueous-phase samples in contact with different types of soil, which enabled the calculation of distribution coefficient values. Our work shows that remifentanil is strongly bound to all of the soil types that we studied. The primary remifentanil hydrolysis product (R26) was detected in extracts from each soil type. In each case, it appeared that a low level of R26 formed relatively quickly. These results indicate that remifentanil is relatively stable in low pH water and moist soil types and is immobile in a soil environment.

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Document Details

Document Type
Technical Report
Publication Date
Aug 14, 2019
Accession Number
AD1078500

Entities

People

  • Ai K. Sohrabi
  • Bruce E. King
  • Morgan Minyard
  • Roberta Xega

Tags

Communities of Interest

  • Counter WMD

DTIC Thesaurus Topics

  • Chemical Kinetics
  • Chemical Synthesis
  • Chemistry
  • Chromatography
  • Coefficients
  • Detection
  • Electrospray Ionization
  • Environment
  • Groundwater
  • Kinetics
  • Liquid Chromatography
  • Liquid Phases
  • Liquids
  • Mass Spectrometry
  • Recovery
  • Solid Phases
  • Spectrometry

Readers

  • Analytical Chemistry
  • Clinical Trial Research.
  • Groundwater Contamination Remediation.