Cubic Nonlinearity of Transition Metal Dichalcogenides in Atomic Layers for Defense Applications

Abstract

Major Goals: The major goals of project were: 1) to characterize the cubic nonlinearity of 2-dimensional (2D) transition metal dichalcogenides (TMDCs, MX2; M=Mo or W; X=S and Se) atomic layers for DoDs nonlinear photonic applications; 2) to train the number of graduate and undergraduate students in emerging technologies related to the 2D atomic layers; and 3) to strengthen the pipeline of good students pursuing advanced degrees in science and technology through outreach activities involving local and regional schools. Accomplishments: The following activities are accomplished under the goal during the reporting period: Material preparation of mechanically exfoliated atomic layers of two-dimensional transition metal dichalcogenides (TMDCs, MX2; M: Mo or W; X: S or Se) on Si-wafer, sapphire window, and liquid suspension for Z-scan and spatial self-phase modulation. Study of cubic nonlinearity of TMDC atomic layer using the open and closed Z-scan and spatial self-phase modulation as functions of applied intensities and sample positions. The characterization includes: (1) nonlinear transmittance as functions of the sample positions in open z-scan for different excitation intensities; (2) nonlinear transmittance as functions of the sample positions in closed z-scan for different excitation intensities; (3) the magnitude and polarity of third-order nonlinearity; (4) nonlinear transmittance as a functions of the input intensity (I-scan) at the focal plane of open Z-scan, and the valley and peak positions of nonlinear transmittance in closed Z-scan for the potential applications of optical modulator and photonic devices; and (5) magnitudes and polarities of cubic nonlinearities of atomic layer liquid suspensions. Analyses of exciton polarization dephasing time of tungsten diselenide (WSe2) atomic layer.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Nov 20, 2019
Accession Number
AD1096066

Entities

People

  • Felix Jaetae Seo

Organizations

  • Hampton University

Tags

Communities of Interest

  • Advanced Electronics
  • Biomedical
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Band Structures
  • Chemistry
  • Diffraction
  • Distortion
  • Energy Bands
  • Laser Science
  • Laser Spectroscopy
  • Lasers
  • Materials Science
  • Optical Properties
  • Optics
  • Physics Laboratories
  • Refraction
  • Scattering
  • Spectroscopy
  • Spin-Orbit Interaction
  • Two Dimensional

Fields of Study

  • Physics

Readers

  • Atmospheric Remote Sensing.
  • Materials Science and Engineering.
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene