Isotope Energy Release and Deposition Characteristics in Betavoltaic Materials

Abstract

A Monte Carlo nuclear scattering code Monte Carlo n-particle extended (MCNPX)has been used to calculate electron energy losses in liquid-form radioisotope (RI) layers deposited on the surface of wide-bandgap semiconductor PIN junctions. The RI medium self-attenuation limits the RI layer thickness that is practical to deposit on the surface in order to achieve maximum electrical power output. The optimized RI layer thickness is defined here as the thickness that generates electrical power at 90 of the maximum energy transferrable to an underlying semiconductor layer. Liquid form isotope formats are evaluated using the optimal thickness approach as defined. It is found that for liquid form isotopes of 3 H, 63 Ni, 147 Pm, and 90 Sr, the optimal thicknesses are 2, 15, 50, and 250 m thick, respectively. These results can vary in practice because of recrystallization rate and humidity uptake in the liquid form RI over time, but are useful for design of prototypes, basis for material comparison, and providing guidance for future experimental goals. This evaluation is expected to serve as a reference that enables predictions in future design of stacked volumetric power sources.

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Document Details

Document Type
Technical Report
Publication Date
Apr 01, 2020
Accession Number
AD1096605

Entities

People

  • Brenda Smith
  • Claude Pullen
  • Iain Kierzewski
  • Johnny Russo
  • Marc Litz
  • Mohamed Doumbia
  • Randy Tompkins
  • Stephen Kelley

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Charged Particles
  • Compound Semiconductors
  • Electron Energy
  • Electrons
  • Energy
  • Energy Conversion
  • Energy Storage
  • Energy Transfer
  • Jet Propulsion
  • Materials
  • Nuclear Materials
  • Radioactive Decay
  • Scattering
  • Semiconductors
  • Silicon Carbide
  • Three Dimensional
  • Wide Bandgap Semiconductors

Fields of Study

  • Physics

Readers

  • Aerosol Science/Aerosol Physics
  • Semiconductor Device Technology
  • Solar Photovoltaics and Thermoelectric Devices.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene