Synthesis and Evaluation of Compound 35 as a Potential Botulinum Neurotoxin Inhibitor

Abstract

A pseudotripeptide inhibitor designated as compound 35 was synthesized and tested for its ability to inhibit the catalytic activity of botulinum neurotoxin serotype A (BoNT/A) or serotype B (BoNT/B). Catalytic activity was assessed using a fluorescent microplate assay in which an immobilized substrate for BoNT/A (SNAP-25 peptide) or BoNT/B (synaptobrevin peptide) was released into the medium following addition of the appropriate BoNT light chain (LC). Compound 35 was able to inhibit both LCs with an IC50 of 1 micro M for BoNT/A and 7 micro M for BoNT/B. Compound 35 is the first inhibitor that has been found to be effective against two serotypes of BoNT; these two serotypes are responsible for most human intoxications.

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Document Details

Document Type
Technical Report
Publication Date
Jul 31, 2020
Accession Number
AD1108968

Entities

People

  • Andrew Ternay
  • Heidi Hoard-fruchey
  • James Nicholson
  • Michael Adler

Organizations

  • United States Army Medical Research Institute of Chemical Defense
  • University of Denver

Tags

DTIC Thesaurus Topics

  • Abstracts
  • Alanine
  • Amines
  • Benzoic Acids
  • Biomedical Research
  • Chemical Synthesis
  • Chemistry
  • Chlorides
  • Chromatography
  • Column Chromatography
  • Crystal Structure
  • Electrospray Ionization
  • Equations
  • Inhibition
  • Mass Spectra
  • Mass Spectrometry
  • Muscular Diseases
  • Organic Chemistry
  • Peripheral Nervous System
  • Proteins
  • Silica Gels
  • Spectrometry
  • Standards
  • Therapy

Fields of Study

  • Biology

Readers

  • Microbial Pathology
  • Neurotoxicology