Lithium Compound Characterization via Raman Spectroscopy and Laser-Induced Breakdown Spectroscopy

Abstract

Industries such as lithium-ion battery producers and the nuclear industry community seek to produce and store lithium in pure chemical forms. However, these lithium compounds are reactive with the atmosphere and quickly degrade into less desirable forms. Therefore, industry desires a fast and effective quality control approach to quantify the ingrowth of these secondary lithium chemical forms. This research presents a novel approach using Laser-Induced Breakdown Spectroscopy (LIBS) and Raman spectroscopy in tandem to enhance lithium compound characterization beyond what is achieved by either technique alone. The resulting spectral data are aggregated using data fusion and analyzed using chemometrics for the first time. Additionally, LIBS and Raman spectra are analyzed individually using chemometrics and a comparison is made between the techniques individually and the fused data. It is determined the presence of lithium compounds is best characterized using fused LIBS-Raman data analyzed with partial least squares regression.

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Document Details

Document Type
Technical Report
Publication Date
Mar 01, 2021
Accession Number
AD1145756

Entities

People

  • James T. Stofel

Organizations

  • Air Force Institute of Technology

Tags

Communities of Interest

  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Air Force
  • Chemistry
  • Data Fusion
  • Diffraction
  • Engineering
  • Information Processing
  • Information Science
  • Lasers
  • Light Sources
  • Lithium Compounds
  • Raman Spectra
  • Raman Spectroscopy
  • Scattering
  • Spectra
  • Spectroscopy
  • Two Dimensional
  • X-Ray Diffraction

Readers

  • Battery Technology and Engineering
  • Pulsed Power and Plasma Physics.
  • Systems Analysis and Design

Technology Areas

  • Directed Energy