Selectively Strippable Silyl-Containing Aerospace Topcoats Using Environmentally Friendly Fluoride Salts

Abstract

The polyurethane topcoats used on the exterior of DoD aircraft and ground support equipment (GSE) are removed with hazardous chemical strippers, such as methylene chloride, abrasive materials, such as blast media and sand paper, or thermal ablation. However, all of these methods also damage the underlying non-metallic substrate (e.g. anti-corrosive epoxy primer, carbon fiber reinforced composite) upon removal of the topcoat. Furthermore, a chemical stripper that is environmentally friendly, can selectively remove the polyurethane topcoat with minimal applications, and will not damaging the underlying non-metallic substrate does not currently exist. Herein, we have successfully demonstrated, as a proof-of-concept, that stimuli-responsive silyl-containing polyurethane (Silyl-PU) coatings can provide similar thermal, mechanical, and performance properties (e.g. up to 60 GE Impact flexibility) as a MIL-PRF-85285 qualified polyurethane topcoat, yet also be selectively and completely removed (within 20 minutes) from a strongly adhered epoxy primer using an environmentally friendly fluoride salt solution under mild conditions at room temperature. Removal of the topcoat did not affect the chemical structure of the epoxy primer according to infrared analysis. The Silyl-PU technology, as a topcoat on aircraft, could prevent exposure of hazardous materials (e.g. hexavalent chromium based epoxy primer) to workers and the environment by maintaining an intact primer upon selective removal of the topcoat, thereby reducing costs associated with hazardous waste disposal and reapplication of the primer.

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Document Details

Document Type
Technical Report
Publication Date
Nov 03, 2021
Accession Number
AD1152349

Entities

People

  • Erick B. Iezzi
  • Eugene Camerino
  • Grant C. Daniels
  • Keith B. Sutyak

Organizations

  • United States Naval Research Laboratory

Tags

Communities of Interest

  • Air Platforms
  • Biomedical
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Aircrafts
  • Alcohols
  • Chemical Synthesis
  • Chemistry
  • Chlorides
  • Column Chromatography
  • Fiber Reinforced Composites
  • Glass Transition Temperature
  • Mass Spectrometry
  • Material Degradation Processes
  • Materials
  • Materials Laboratories
  • Materials Processing
  • Materials Science
  • Materials Testing
  • Organic Chemistry
  • Tensile Strength
  • Test Methods
  • Transition Temperature

Fields of Study

  • Materials science

Readers

  • Environmental Engineering.
  • Surface Coatings Technology.

Technology Areas

  • Space