Quantification of In Situ Chemical Reductive Defluorination (ISCRD) of Perfluoroalkyl Acids in Groundwater Impacted by AFFFs

Abstract

At the start of this ER-2426 project, the primary approach to mitigate PFAS transport and contamination of drinking water was sorbents, which came with challenges to effectively capture shorter chain PFAAs. Longevity and regeneration. The primary goal of this project was to identify reductive technologies amenable for in situ destructive remediation of PFAS with PFOS as the initial focus. This research led to the development of a reductive technology using Ni0Fe0 nanoparticles synthesized onto an activated carbon (AC). The technology was demonstrated in batch and 1-D column reactors to transform and mineralize Land br-PFAS with fluoride and sometimes sulfite generation and organic intermediates. All PFAS transformed and mineralized to varying degrees. Additional column studies, which best mimic how well this technology may work in the field either as an in situ permeable reactive barrier, above ground treatment (a reactive GAC rather than just a sorptive GAC) or in situ injection are needed to evaluate further transformation and defluorination at increased residence times.

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Document Details

Document Type
Technical Report
Publication Date
Apr 23, 2021
Accession Number
AD1154408

Entities

People

  • Linda S Lee
  • Loring Nies
  • Victor Medina

Organizations

  • Purdue University

Tags

Communities of Interest

  • Biomedical
  • Energy and Power Technologies
  • Ground and Sea Platforms

DTIC Thesaurus Topics

  • Air Force
  • Air Force Facilities
  • Buffers (Chemistry)
  • Carboxylic Acids
  • Chemical Kinetics
  • Chemical Synthesis
  • Chemistry
  • Department Of Defense
  • Electrospray Ionization
  • Groundwater
  • Hydroxides
  • Ionization
  • Liquid Chromatography
  • Mass Spectrometry
  • Materials
  • Nanoparticles
  • Organic Chemistry
  • Spectra
  • Three Dimensional

Fields of Study

  • Environmental science

Readers

  • Agricultural Chemistry/Soil Science
  • Distributed Systems and Data Platform Development
  • Internal Combustion Engine (ICE) Technology.

Technology Areas

  • Biotechnology
  • Biotechnology - Bioremediation